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| Àâòîðèçàöèÿ |
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| Ïîèñê ïî óêàçàòåëÿì |
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| Mukamel S. — Principles of nonlinear spectroscopy |
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| Ïðåäìåòíûé óêàçàòåëü |
Optical measurements, interpretation of 111
Optical measurements, polarization and 93—103
Optical polarization 3 111 129 151
Optical polarization in macroscopic system 128
Optical polarization, anharmonic oscillator picture 163—167
Optical polarization, calculation of 111 113
Optical polarization, dispersive in-phase contribution see Birefringence
Optical processes, classification, by power-law dependence 3—5 4f
Optical processes, classification, by resonant mode 7 9—10 10f—12f 12—13
Optical processes, classification, by temporal profile 5f—7f 5—7
Optical processes, frequency-domain 127
Optical response functions of extended systems, nonlocal expressions for 123—124
Optical response functions of homogeneous medium of noninteracting particles 127—128
Optical response functions of multilevel system with relaxation 143—144 149—151 152f—158f 153—159
Optical response functions of multilevel system with relaxation, Kramers — Kronig relations and 144—146 147f
Optical response functions of multilevel system with relaxation, linear response in Liouville space and 147—149
Optical response functions, semiclassical simulation 187—188
Optical response functions, simulations, coherence Green function and 203 204—205
Optical response functions, simulations, equation derivation for 206—207
Optical response functions, simulations, moments of linear absorption and 193—196 195f
Optical response functions, simulations, phase averaging and 189f 189—192 199—201
Optical response functions, simulations, static limit of 201—203
Optical spectroscopy, vs. nuclear magnetic resonance 12
Optical Stark effect 446 514
Optical susceptibilities 124 127 150 171 244 245 445 466
Optical susceptibilities of multilevel system interacting with medium in arbitrary timescale 244—247
Optical susceptibilities of periodic structures in k space 496—498
Optical susceptibilities, linear 95 128 145
Optical susceptibilities, linear, real and imaginary parts 152f
Optical susceptibilities, local field expressions of homogeneous systems 475—477
Optical susceptibilities, nonlinear 12 151 157 462 479
Optical susceptibilities, nonlinear, enhanced, in molecular aggregates 498—504 503f—506f 506—507
Optical susceptibilities, nonlinear, exciton-population variables and 507—512 511f—512f
Optical susceptibilities, second-order 128
Optical susceptibilities, third-order 128 162
Ordinary rate equation 184
Orthogonality in Hilbert space vs. Liouville space 58f
Orthogonality, scalar product rule for 42
Orthonormality 50 56
Oscillator strength sum rule 165
Oscillators, continuous distribution of 221—226 225f 226f
Oscillators, harmonic 17 163 164 233
Out-of-phase polarization 446
Outer product of vectors in Hilbert space 41 56
Outer product of vectors in Liouville space 57
Overdamped motions, strongly 333
Pade approximant 225
Particle dynamics 386—387
Particle velocity 88
Path integral in Liouville space 349
Path integral, techniques 227
Pauli anticommutation rule 470
Pauli exclusion principle, Bloch equations and 491
Pauli exclusion principle, definition of 471
Pauli exclusion principle, enhanced nonlinear susceptibilities in molecular aggregates and 513—514
Pauli exclusion principle, Frenkel exciton model and 499 502
Pauli exclusion principle, Green function expression and 487
Pauli exclusion principle, pure state factorization and 489
PE (two-pulse photon echo) 295
Pentacene, fluorescence excitation spectrum 291f
Pentacene, spectral diffusion 389f
Permutations over fields 124 125
Perturbation series, partial resummation of 30
Perturbation theory 27
Perturbative expansion 116
Perturber, effect on linear absorption 238
Phase conjugation 175
Phase matching condition 98 98f
Phase relaxation see Dephasing
Phase shift, in binary collision 238
Phase space 69 71—72 75
Phase space, filling 491
Phase-averaging 349—351
Phase-averaging in Liouville space 199—201
Phase-locked pump-probe absorption, three-pulse 338—339
Phase-locked spontaneous light emission spectroscopy (PLSLE) 295 310—312 340 341
Phase-locked transient gratings 324 324f 325f 326
Phase-sensitive detection 99
Phonons 514
Photon echo spectroscopy 4 99 133 295 432 474
Photon echo spectroscopy, accumulated, unified theory for 295 314—315
Photon echo spectroscopy, accumulated, unified theory for, with incoherent light sources 316—317
Photon echo spectroscopy, impulsive 301—304 302f
Photon echo spectroscopy, impulsive, Brownian oscillator analysis of 304—306 307f—310f 308 310
Photon echo spectroscopy, term, use of 304
Photon echo spectroscopy, three-pulse 295
Photon echo spectroscopy, three-pulse, with homodyne or heterodyne detection 299—301 300f
Photon echo spectroscopy, two-pulse 301
Photon emission rate 265 266
Physical  function 129
PIC (pseudoisocyanine bromide) 491 504f 505f
Picosecond pulse shaping techniques 423
Picosecond Raman spectroscopy 413 417—418 430—431
PIER 4 (pressure-induced extra resonance in four-wave mixing) 282
Planck’s constant 16
PLSLE (phase locked spontaneous light emission spectroscopy) 295 310—312 340 341
Poisson bracket 70 257
Poisson distribution 220
Polar medium, dielectric fluctuations, cumulant expansion and 234 236—237
Polariton 515f 515
Polarizability 122 124
Polarizability of molecular assemblies linear 495
Polarizability of molecular assemblies third-order 492 496
Polarizability operator 416
Polarizability, autocorrelation function 199
Polarization 79 83 92 113 164 445—446
Polarization, density 87 87f 93 112 127
Polarization, linear 3
Polarization, multipolar expansion of 83 106—107
Polarization, nonlinear response functions, rotational contribution to 447—450
Polarization, operator 82 84 123 160
Polarization, operator, microscopic definition of 82—83 111
Polarization, optical measurements and 93—103
Polarization, optical measurements and, absorption of weak probe 100—103
Polarization, optical measurements and, heterodyne detection of wave mixing 99—100
Polarization, optical measurements and, linear absorption 94—96
Polarization, optical measurements and, multiwave mixing 96—99 98f
Polarization, polarization-dependent grating signal 451—455 454f 455f
Polarization, scalar product 87
Polarization, second-order 159
Polarization, third-order 4 116 159 433 446 496
Polarization, third-order, nonlinear techniques see Off-resonance spectroscopy
Polarization, time-dependent 115
Polarization, vector field 85
Polarization, vector, third-order 447—448
Polarization, vibrational contribution to heterodyne-detected transient grating 450—451
Polarization-sensitive techniques 445
Population relaxation 176 181
Population relaxation and pure dephasing 516—517
Population relaxation, matrix 144
Population relaxation, realistic,  with 167—169 168f
Populations 47 134
Populations, damping of 134
Populations, time-dependent 52—53
Positive time ordered exponential 24
Power law, dependence, optical measurements and 3—5
Power — Zienau transformation 84—88 87f
Poynting vector 90
Pressure broadening (collisional broadening) 238
Pressure-induced extra resonance in four-wave mixing (PIER 4) 282
Principal part of integral 38
Probability, conservation of 178 182
Probe absorption for snapshot spectrum 377—382
Probe absorption, field and matter perspective 101—102
Probe difference absorption 327
Probe field amplitude 103
Product of operators, normally ordered 485
Product of operators, trace of 46
Projection operators 177
Projection operators in Liouville space 67—68
| Projection operators, definition of 34—35
Projection operators, idempotent 35
Propagation 144
Pseudoisocyanine bromide (PIC) 491 504f 505f
PTCDA (3,4,9,10-perylenetetracarboxylic dianhydride) 480f
Pulse shaping 414
Pump-probe spectroscopy 360 369 376 445
Pump-probe spectroscopy in three-electronic-level system 393—394 394f
Pump-probe spectroscopy in three-electronic-level system, coherent vs. sequential components of 395—396
Pump-probe spectroscopy in three-electronic-level system, interplay of field and matter coherence 399—403
Pump-probe spectroscopy in three-electronic-level system, snapshot limit for 396—399 398f—401f
Pump-probe spectroscopy of GaAs quantum well 370f
Pump-probe spectroscopy, absorption 7 8f
Pump-probe spectroscopy, classical limit 385
Pump-probe spectroscopy, detuning 9f
Pump-probe spectroscopy, doorway-window picture 133
Pump-probe spectroscopy, doorway-window picture, time variables for 375f
Pump-probe spectroscopy, formal expression 373
Pump-probe spectroscopy, Fourier transform relationship with hole-burning 340—343 342f
Pump-probe spectroscopy, impulsive 414
Pump-probe spectroscopy, impulsive, homogeneous broadening limit 335
Pump-probe spectroscopy, impulsive, inhomogeneous broadening and 294 333 335
Pump-probe spectroscopy, impulsive, quantum beats and 328—333 329f—331f 334f 335 335f
Pump-probe spectroscopy, long pulses, vs. electronic dephasing 382—383
Pump-probe spectroscopy, off-resonance 384—385
Pump-probe spectroscopy, phase locking in 312
Pump-probe spectroscopy, phase-locked transient grating and 324
Pump-probe spectroscopy, quantum beats 294—295 305
Pump-probe spectroscopy, resonant impulsive pump 383—384
Pump-probe spectroscopy, sequential 322 326—328 327f 336
Pump-probe spectroscopy, short pulses, vs. nuclear dynamics 382
Pump-probe spectroscopy, short pulses, vs. nuclear dynamics and long vs. electronic dephasing 377—382
Pump-probe spectroscopy, signal generation 4—5
Pump-probe spectroscopy, snapshot spectrum 377—382
Pump-probe spectroscopy, third-order polarization and 116
Pump-probe spectroscopy, time-domain 380
Pump-probe spectroscopy, two-photon absorption 173
Pump-probe spectroscopy, with frequency dispersed detection, wavepacket representation of 407
Pure dephasing 516—517
Pure dephasing and population relaxation 516—517
Pure dephasing, Green function for 519
Pure dephasing, processes 161 179—180
Pure dephasing, rate 149 169 179 187 310 310f
Pure dephasing, relaxation times 181
Pure state 47 49t 52 136 159
Quadratic detection see Homodyne detection
Quantized transverse electromagnetic field 81
Quantum beats 5 305 333 369 420
Quantum beats, impulsive pump limit and 369
Quantum beats, impulsive pump-probe spectroscopy and 328—333 329f—331f 334f 335 335f
Quantum dynamics in Hilbert space see Hilbert space
Quantum dynamics in Liouville space see Liouville space
Quantum electrodynamics, coupled Maxwell — Liouville equations 92—93
Quantum electrodynamics, electrostatic intermolecular interaction and 86—88 87f
Quantum electrodynamics, equations of motion for field 89—90
Quantum electrodynamics, minimal (p.A.) coupling Hamiltonian and 79—84
Quantum electrodynamics, multipolar Hamiltonian and 85—86
Quantum electrodynamics, power-Zienau transformation and 84—85
Quantum electrodynamics, radiation-matter interaction and 79—83
Quantum electrodynamics, semiclassical material equations 90—92
Quantum field, absorption of 262—264 263f
Quantum harmonic oscillator, Hamiltonian for, in Wigner representation 73 74f
Quantum Liouville equation 51
Quantum mechanical average 494
Quantum theory of relaxation 53
Quantum wells 479—480
Quantum wires 479—480
Rabi formula 20
Rabi frequency 20
Rabi oscillations 20—21 183
Radiation fields 114
Radiation fields, degrees of freedom 23
Radiation fields, perturbative expansion 112
Radiation fields, retardation effects 112
Radiation fields, vacuum fluctuations of 261
Radiation fields, weak field approach 112
Radiation-matter interaction 264
Radiation-matter interaction, minimal coupling Hamiltonian and 79—83
Radiation-matter interaction, quantum description of 112 155—156
Radiation-matter interaction, time-dependent 29
Radiative decay 513
Raman excitation, filtering effect using pulse shaping 428
Raman polarization 413
Raman resonance 411
Raman spectroscopy 170 261—262 262f 263f 361
Raman spectroscopy, femtosecond 294 417—418 428
Raman spectroscopy, fluorescence and 271—279 272f 274f—279f
Raman spectroscopy, inhomogeneous broadening and 294
Raman spectroscopy, off-resonant conditions 10
Raman spectroscopy, picosecond 413 417—418 430—431
Raman spectroscopy, probe field in 453
Raman spectroscopy, stationary 294
Raman spectroscopy, timescales for 412
Raman spectroscopy, two-dimensional 435—436
Reduced density operator 134 356
Reduced description 132
Reduced doorway wavepacket 429
Reduced equations of motion, for Liouville space wavepackets 357—359
Reference frequency for spectral moments 193 194
Reference nuclear configuration 210
Reflection 3 144
Refraction 3 144
Relaxation 12 131
Relaxation of population 177—178
Relaxation, homogeneous broadening 169
Relaxation, inhomogeneous broadening 169
Relaxation, matrix, conservation of probability and 178
Relaxation, matrix, criteria for 178
Relaxation, model 168
Relaxation, rates 38 143 230
Relaxation, superoperator 68 163 179
Relaxation, superoperator, calculation 144 176—180
Relaxed fluorescence 250
Relaxed fluorescence, lineshapes 233f
Relaxed fluorescence, spectrum 220 220f
Relevant polarization 130
Renormalized perturbation theory 162
Resonance frequency 151
Resonant coherent Raman spectroscopy 279—285 280f 284f see
Resonant fluorescence anisotropy 446
Resonant gratings 321—322
Resonant impulsive pump 383—384
Resonant techniques see also Specific resonant techniques
Resonant techniques vs. off-resonant techniques 7 9—10 10f—12f 12—13
Resorufin, absorption and emission spectra 308 308f
Resorufin, photon echo signal 308 309f
Response functions 112
Response functions of multilevel manifold with relaxation 149—151 152f—158f 153—159
Response functions of two-level model 209
Response functions, calculation methods 209
Response functions, classical correlation functions and 242 257—258
Response functions, linear 94 150
Response functions, nth-order 445
Response functions, second-order 150 170—171
Response functions, second-order, cumulant expansion 213
Response functions, second-order, Liouville space coupling for 156f
Response functions, semiclassical expansion 211
Response functions, single-particle, macroscopic susceptibilities and 127
Response functions, small particle, correlation function expressions for 111—118 115f
Response functions, third-order 150 203 210
Response functions, third-order, cumulant expansion 213
Response functions, third-order, Hilbert vs. Liouville space representation of 196—199 197f
Response functions, wavevector dependence of 112
Rhodamine, fluorescence excitation spectrum 194 195f
Rhodopsin, isomerization dynamics 370f
Rigid rotor 17
Rontgen current 90
Rotating wave approximation (RWA) 296 366 375 411 418 446 495
Rotating wave approximation for coherent anti-Stokes Raman spectroscopy 281 285
Rotating wave approximation, Bloch equations and 169 181 183
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