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Derjaguin B.V., Prokhorov A.V., Tunitskij N.N. — Statistical Thermodynamics of the Formation of a New Phase in the Boiling Up of Volatile Liquids
Derjaguin B.V., Prokhorov A.V., Tunitskij N.N. — Statistical Thermodynamics of the  Formation of a New Phase in the Boiling Up of Volatile Liquids



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Название: Statistical Thermodynamics of the Formation of a New Phase in the Boiling Up of Volatile Liquids

Авторы: Derjaguin B.V., Prokhorov A.V., Tunitskij N.N.

Аннотация:

Journal of Statistical Physics, Vol. 23, No. 4, 1980. p. 495-520.
The fluctuation growth of a macroscopic bubble containing a vapor in a moderately superheated or tensile-stressed volatile liquid is treated as the two-dimensional diffusion of a nucleus of a new phase in the space of variables made up of its volume v and the pressure of the vapor in it p. The shape of the free energy surface of the system "liquid plus bubble with vapor" in the plane (v; p) in the neighborhood of the labile equilibrium of the system is examined, and a two-dimensional nucleus distribution function given with respect to its variables is derived. Close to the pass in the surface a nondiagonal diffusion tensor in the space (v, p) is also calculated. A two-dimensional stationary equation of the kinetics of the formation of a new phase of Kramers type is solved, and an expression is derived for the probability of homogeneous nucleation for an arbitrary viscosity and volatility of a liquid far from its critical point. Various limiting cases are examined.


Язык: en

Рубрика: Физика/

Тип: Статья

Статус предметного указателя: Неизвестно

ed2k: ed2k stats

Год издания: 1980

Количество страниц: 26

Добавлена в каталог: 29.09.2013

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